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[40] Plasmonic Activity of Large-Area Gold-Nanodot Arrays on Arbitrary Substrates

01

Nov

2009

Typical top view of a large area gold nanodot matrix on a sapphire substrate made by DiMPLA. Three-dimensional view (radius = 300 nm) of the simulated optical response of an isolated, semisubmersed Au sphere (radius = 84 nm). The quarter cutaway reveals the Au−sapphire and sapphire−air interface geometries. The same color scale as in (b) indicates the scattered |Ez| component for λexc = 942 nm at normal incidence.

Nano Lett. 2010, 10 (1), pp 47–51
Link to paper

Marisa Mäder, Thomas Höche*, Jürgen W. Gerlach, Susanne Perlt, Jens Dorfmüller, Michael Saliba, Ralf Vogelgesang, Klaus Kern and Bernd Rauschenbach
Leibniz Institute of Surface Modification, Permoserstrasse 15, D-04318 Leipzig, Germany
Max-Planck-Institute for Solid State Research, Heisenbergstrasse 1, D-70569 Stuttgart, Germany
Nano Lett., 2010, 10 (1), pp 47–51
DOI: 10.1021/nl903633z
Publication Date (Web): December 16, 2009
Copyright © 2009 American Chemical Society
Abstract. Highly efficient fabrication of well-ordered, embedded gold nanodot matrices using diffraction mask projection laser ablation is demonstrated. These gold nanodot arrays are ideally generated onto sapphire substrates but do also form onto AlOx thin films, enabling the application to arbitrary bulk substrates. Well-ordered gold dots become embedded into the Al2O3 substrate during the process, thus improving their mechanical stability, chemical inertness, and technological compliance. Such substrates may be useful, for example, to enhance solar-cell efficiency by surface plasmons or as convenient, biocompatible focusing elements in nearfield optical tweezers.